Metal–Organic‐Framework‐Derived Carbons: Applications as Solid‐Base Catalyst and Support for Pd Nanoparticles in Tandem Catalysis

dc.contributor.author Li, Xinle
dc.contributor.author Zhang, Biying
dc.contributor.author Fang, Yuhui
dc.contributor.author Sun, Weijun
dc.contributor.author Huang, Wenyu
dc.contributor.author Qi, Zhiyuan
dc.contributor.author Pei, Yuchen
dc.contributor.author Qi, Shuyan
dc.contributor.author Yuan, Pengyu
dc.contributor.author Luan, Xuechen
dc.contributor.author Goh, Tian Wei
dc.contributor.author Huang, Wenyu
dc.contributor.department Ames Laboratory
dc.contributor.department Mechanical Engineering
dc.contributor.department Chemistry
dc.date 2018-06-30T08:08:46.000
dc.date.accessioned 2020-06-30T01:16:05Z
dc.date.available 2020-06-30T01:16:05Z
dc.date.copyright Sun Jan 01 00:00:00 UTC 2017
dc.date.issued 2017-03-29
dc.description.abstract <p>The facile pyrolysis of a bipyridyl metal‐organic framework, MOF‐253, produces N‐doped porous carbons (Cz‐MOF‐253), which exhibit excellent catalytic activity in the Knoevenagel condensation reaction and outperform other nitrogen‐containing MOF‐derived carbons. More importantly, by virtue of their high Lewis basicity and porous nature, Cz‐MOF‐253‐supported Pd nanoparticles (Pd/Cz‐MOF‐253‐800) show excellent performance in a one‐pot sequential Knoevenagel condensation‐hydrogenation reaction.</p>
dc.description.comments <p>This is the peer-reviewed version of the following article: Li, Xinle, Biying Zhang, Yuhui Fang, Weijun Sun, Zhiyuan Qi, Yuchen Pei, Shuyan Qi et al. "Metal–Organic‐Framework‐Derived Carbons: Applications as Solid‐Base Catalyst and Support for Pd Nanoparticles in Tandem Catalysis." <em>Chemistry-A European Journal</em> 23, no. 18 (2017): 4266-4270, which has been published in final form at doi: <a href="http://dx.doi.org/10.1002/chem.201605852" target="_blank">10.1002/chem.201605852</a>. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Self-Archiving. Posted with permission.</p>
dc.format.mimetype application/pdf
dc.identifier archive/lib.dr.iastate.edu/chem_pubs/1028/
dc.identifier.articleid 2030
dc.identifier.contextkey 12402002
dc.identifier.s3bucket isulib-bepress-aws-west
dc.identifier.submissionpath chem_pubs/1028
dc.identifier.uri https://dr.lib.iastate.edu/handle/20.500.12876/14324
dc.language.iso en
dc.source.bitstream archive/lib.dr.iastate.edu/chem_pubs/1028/2017_Huang_MetalOrganic.pdf|||Fri Jan 14 18:17:27 UTC 2022
dc.source.uri 10.1002/chem.201605852
dc.subject.disciplines Chemistry
dc.subject.disciplines Materials Chemistry
dc.subject.disciplines Mechanics of Materials
dc.subject.keywords Knoevenagel condensation
dc.subject.keywords metal–organic frameworks
dc.subject.keywords n-doped carbons
dc.subject.keywords palladium
dc.subject.keywords tandem catalysis
dc.title Metal–Organic‐Framework‐Derived Carbons: Applications as Solid‐Base Catalyst and Support for Pd Nanoparticles in Tandem Catalysis
dc.type article
dc.type.genre article
dspace.entity.type Publication
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